It would be possible, even easy.
In gui.c, just replace
static const char* modes[]={ "Off", "1/3 EV","2/3 EV", "1 EV", "1 1/3Ev", "1 2/3Ev", "2 Ev"};
with
static const char* modes[]={ "Off", "1/3 EV","2/3 EV", "1 EV", "1 1/3Ev", "1 2/3Ev", "2 Ev", "2 1/3Ev", "2 2/3Ev", "3 Ev", "3 1/3Ev", "3 2/3Ev", "4 Ev"};
just after
const char* gui_tv_bracket_values_enum(int change, int arg) {
and
const char* gui_av_bracket_values_enum(int change, int arg) {